Year: 2003
Type: article
Abstract: The fluctuation–dissipation relation is measured on the dielectric properties of a gel (Laponite) and of a polymer glass (polycarbonate). For the gel it is found that during the transition from a fluid-like to a solid-like state the fluctuation–dissipation theorem is strongly violated. The amplitude and the persistence time of this violation are decreasing functions of frequency. Around 1 Hz it may persist for several hours. A very similar behaviour is observed in polycarbonate after a quench below the glass transition temperature. In both cases the origin of this violation is a highly intermittent dynamics characterized by large fluctuations. The relevance of these results for recent models of ageing is discussed.
Authors: L Buisson, L Bellon, S Ciliberto
Language: English
Subfield: Materials Chemistry
Field: Materials Science
Domain: Physical Sciences
Open Access status: bronze
OpenAlex ID: W2064936892
