Year: 2009
Type: article
Abstract: An exact and nonperturbative quantum master equation can be constructed via the calculus on the path integral. It results in hierarchical equations of motion for the reduced density operator. Involved also are a set of well-defined auxiliary density operators that resolve not just the system–bath coupling strength but also memory. In this work, we scale these auxiliary operators individually to achieve a uniform error tolerance, as set by the reduced density operator. An efficient propagator is then proposed to the hierarchical Liouville-space dynamics of quantum dissipation. Numerically exact studies are carried out on the dephasing effect on population transfer in the simple stimulated Raman adiabatic passage scheme. We also make assessments on several perturbative theories for their applicabilities in the present system of study.
Source: New Journal of Physics
Authors: Jian Xu, Rui-Xue Xu, Yi Jing Yan
Language: English
Subfield: Atomic and Molecular Physics, and Optics
Field: Physics and Astronomy
Domain: Physical Sciences
Open Access status: gold
Estimated APC paid: $2,610
OpenAlex ID: W2134113634