Retrieving the susceptibility from time-resolved terahertz experiments
Year: 2007
Type: article
Abstract: We present an analytical expression for the observed signal in time- and phase-resolved pump-probe studies, with particular emphasis on terahertz time-domain spectroscopy. Maxwell's equations are solved for the response of damped, harmonic oscillators to a driving probe field in the perturbative regime. Our analytical expressions agree with the one previously reported in the literature [Nemec et al., J. Chem. Phys. 122, 104503 (2005)] in the Drude limit; however, they differ in the case of a vibrational resonance.
Source: The Journal of Chemical Physics
DOI: 10.1063/1.2761915
Authors: J. M. Schins, E. Hendry, M. Bonn, H. G. Muller
Language: English
Subfield: Electrical and Electronic Engineering
Field: Engineering
Domain: Physical Sciences
Open Access status: green
OpenAlex ID: W2160112769
