Work

Network theory for inhomogeneous thermoelectrics

Year: 2016
Type: article
Abstract: The Onsager–de Groot–Callen transport theory, implemented as a network model, is used to simulate the transient Harman method, which is widely used experimentally to determine all thermoelectric transport coefficients in a single measurement setup. It is shown that this method systematically overestimates the Seebeck coefficient for samples composed of two different materials. As a consequence, the figure of merit is also overestimated, if the thermal coupling of the measurement setup to the environment is weak. For a mixture of metal and semiconductor particles near metal percolation the figure of merit obtained by the Harman method is more than 100% too large. For a correct interpretation of the experimental data, information on composition and microstructure of the sample are indispensable.
Authors: Sebastian Angst, Dietrich E Wolf
Language: English
Open Access status: gold
Estimated APC paid: $2,610
Award: G757383574
OpenAlex ID: W2282435648
FWCI: 0.513
Cites: 33
Cited by: 10
Related to: 10