Work

The pursuit of commercial silicon-based microparticle anodes for advanced lithium-ion batteries: A review

Year: 2022
Type: review
Abstract: Silicon (Si) is one of the most promising anode materials for high-energy lithium-ion batteries. However, the widespread application of Si-based anodes is inhibited by large volume change, unstable solid electrolyte interphase, and poor electrical conductivity. During the past decade, significant efforts have been made to overcome these major challenges toward industrial applications. This review summarizes the recent development of microscale Si-based electrodes fabricated by Si microparticles or other industrial bulk materials from the perspective of industrialization. First, the challenges for microscale Si anodes are clarified. Second, structural design strategies of stable micro-sized Si materials are discussed. Third, other critical practical metrics, such as robust binder construction and electrolyte design, are also highlighted. Finally, future trends and perspectives on the commercialization of Si-based anodes are provided.
Language: English
Open Access status: diamond
OpenAlex ID: W4306367217
FWCI: 1.47
Cites: 184
Cited by: 113
Related to: 10