Year: 2024
Type: article
Abstract: We report on the microscopic superconducting properties of the Dirac semimetal ${\mathrm{PdTe}}_{2}$. In this study, we have focused on mosaic crystals of ${\mathrm{PdTe}}_{2}$, and used detailed zero-field and transverse-field muon-spin relaxation/rotation $(\ensuremath{\mu}\mathrm{SR})$, ac-magnetic susceptibility, and resistivity measurements to investigate their superconducting properties. The magnetic susceptibility measurements reveal two superconducting transition temperatures at 1.8 and 1.6 K, respectively, in agreement with earlier reports. In contrary to these reports, we find that these mosaic ${\mathrm{PdTe}}_{2}$ crystals are not type-I, but rather type-II superconductors. In fact, we observe the clear manifestation of a flux-line lattice through a clear diamagnetic shift and Gaussian broadening of the Fourier spectra in the superconducting state. This behavior is likely caused by the disorder in the mosaic crystals of ${\mathrm{PdTe}}_{2}$ studied here. Our analysis of the superconducting order parameter by the means of temperature-dependent magnetic penetration depth $\ensuremath{\lambda}(T)$ reveals a fully gapped superconducting state that can be well-fitted using an $s$-wave symmetric gap. We find that ${\mathrm{PdTe}}_{2}$ is a promising model system for the investigation and interplay of nontrivial topology, surface superconductivity, and type-II bulk superconductivity in a van der Waals material. Moreover, our results indicate that the superconductivity in this material can be easily modified from type-I to type-II by disorder in the system.
Language: Latvian
Subfield: Condensed Matter Physics
Field: Physics and Astronomy
Domain: Physical Sciences
Open Access status: bronze
Awards: Discovery of Topological Superconductivity by Combining Physical and Chemical Design Principles, Novel Magnetic and Topological 2D Materials (MAGICAL 2D), G2341168950, Charge Density Wave and Superconductivity: Investigation on the Coexistence, Coupling and Competition of the Two Ground States, G993971353
OpenAlex ID: W4394568151
