Year: 2024
Type: article
Abstract: Parametric resonances and amplification have led to extraordinary photoinduced phenomena in pump-probe experiments. While these phenomena manifest themselves in out-of-equilibrium settings, here, we present the striking result of parametric amplification in equilibrium. We demonstrate that quantum and thermal fluctuations of a Raman-active mode amplifies light inside a cavity, at equilibrium, when the Raman mode frequency is twice the cavity mode frequency. This noise-driven amplification leads to the creation of an unusual parametric Raman polariton, intertwining the Raman mode with cavity squeezing fluctuations, with smoking gun signatures in Raman spectroscopy. In the resonant regime, we show the emergence of not only quantum light amplification but also localization and static shift of the Raman mode. Apart from the fundamental interest of equilibrium parametric amplification, our Letter suggests a resonant mechanism for controlling Raman modes and thus matter properties by cavity fluctuations. We conclude by outlining how to compute the Raman-cavity coupling, and suggest possible experimental realizations.
Source: Physical Review Letters
Language: English
Subfield: Atomic and Molecular Physics, and Optics
Field: Physics and Astronomy
Domain: Physical Sciences
Open Access status: green
OpenAlex ID: W4402356232