Work

Design and Development of Integrated Direct Air Capture and Methanation Processes

Year: 2024
Type: article
Abstract: The synergies from integrating direct air capture and CO2 methanation are assessed and quantified. Three direct air capture and methanation processes with different integration strategies are proposed: only heat integration, direct air capture sorbent regeneration with high‐pressure H2, and complete integration in a single unit. The heat integration study via pinch analysis evaluated the potential energy demand reduction. Overall autothermal operation is achievable, as the heat generated in methanation often exceeds that required for direct air capture sorbent regeneration. A novel process combining CO2 adsorption and methanation in one reactor provided the best productivity and energy demand results. However, this design requires complex cycles and strict demands on the sorbent and catalyst, requiring further development and experimental demonstration.
Language: English
Open Access status: hybrid
Estimated APC paid: $3,840
OpenAlex ID: W4403792202
FWCI: 0.948
Cites: 17
Cited by: 7
Related to: 10