Work

Megahertz-rate NO planar laser-induced fluorescence of reacting flows using tunable 5th harmonic Nd:YAG with A-X and B-X excitation

Year: 2025

Type: article

Abstract: This article presents the first demonstration of burst-mode nitric oxide planar laser-induced fluorescence measurement of a reacting environment via Nd:YAG 5th harmonic excitation. A tunable pulse-burst laser generated 1 ms bursts of resonant 213 nm radiation at 200 kHz, 500 kHz, and 1 MHz repetition rates with 16 mJ, 3.5 mJ, and 0.75 mJ average pulse energies, respectively. Nitric oxide, naturally formed in the vicinity of an oxy-acetylene flame, was targetted via three excitation schemes: γ(1,0), γ(1,0) + β(5,1), and β(4,1). The generated fluorescence was collected in two separate spectral windows to demonstrate the selectivity of the electronic excitation and explore new filtering approaches for high background luminosity environments: 240 nm - 260 nm and 275 nm - 375 nm. Overall, this new method of UV-light generation for nitric oxide excitation performed very well with a substantial amount of collected signal even with modest energy levels accessible at a 1 MHz rate. The primary advantage of utilizing the 5th harmonic to access nitric oxide resonances was its simplicity and robustness through direct burst mode laser up-conversion and simplified Master Oscillator, Power Amplified (MOPA) frequency control, obviating the need for an optical parametric oscillator.

Source: Optics Express

DOI: 10.1364/oe.553172

Authors: Boris S. Leonov, Christopher J. Grunbok, Richard B. Miles

Institution: Princeton University

Language: English

Topic: Spectroscopy and Laser Applications

Subfield: Spectroscopy

Field: Chemistry

Domain: Physical Sciences

Open Access status: gold

Estimated APC paid: $2,270

Funder: Office of Naval Research