Dual wavelength Brillouin laser terahertz source stabilized to carbonyl sulfide rotational transition
Year: 2025
Type: article
Abstract: Optical-based terahertz sources are important for many burgeoning scientific and technological applications. Among such applications is precision spectroscopy of molecules, which exhibit rotational transitions at terahertz frequencies. Stemming from precision spectroscopy is frequency discrimination and stabilization of terahertz sources. Because many molecular species exist in the gas phase at room temperature, their transitions are prime candidates for practical terahertz frequency references. We demonstrate the stabilization of a low phase-noise, dual-wavelength Brillouin laser (DWBL) terahertz oscillator to a rotational transition of carbonyl sulfide (OCS). We achieve an instability of $1.2\times10^{-12}/\sqrt{\tau}$, where $\tau$ is the averaging time in seconds. The signal-to-noise ratio and intermodulation limitations of the experiment are also discussed. We thus demonstrate a highly stable and spectrally pure terahertz frequency source. Our presented architecture will likely benefit metrology, spectroscopy, precision terahertz studies, and beyond.
Source: Nature Communications
Authors: James Greenberg, Brendan M. Heffernan, William F. McGrew, Keisuke Nose, Antoine Rolland
Institution: IMRA America (United States)
Language: English
Subfield: Atomic and Molecular Physics, and Optics
Field: Physics and Astronomy
Domain: Physical Sciences
Open Access status: gold
Estimated APC paid: $6,990
OpenAlex ID: W4408307363