Intertwined Superconductivity and Orbital Selectivity in a Three-Orbital Hubbard Model for the Iron Pnictides
Year: 2025
Type: article
Abstract: We study a three-orbital Hubbard-Kanamori model relevant for iron-based superconductors using variational wave functions explicitly including spatial correlations and electron pairing. We span the nonmagnetic sector from filling n=4, which is representative of undoped iron-based superconductors, to n=3, where a Mott insulating state with each orbital at half filling is found. In the strong-coupling regime, when the electron density is increased, we find a spontaneous differentiation between the occupation of d_{xz} and d_{yz} orbitals, leading to an orbital-selective state with a nematic character that becomes stronger at increasing density. One of these orbitals stays half filled for all densities while the other one hosts (together with the d_{xy} orbital) the excess of electron density. Most importantly, in this regime long-range pairing correlations appear in the orbital with the largest occupation. Our results highlight a strong link between orbital-selective correlations, nematicity, and superconductivity, which requires the presence of a significant Hund's coupling.
Source: Physical Review Letters
Language: English
Field: Materials Science
Domain: Physical Sciences
Open Access status: green
OpenAlex ID: W4410364576