Work

Shape-anisotropy inverses the behavior of emergent vortices in active chiral fluids

Year: 2025
Type: article
Abstract: Active colloidal fluids exhibit spontaneous emergence of correlated states, characterized by complex collective dynamics and self-organization. In geometrically confined systems, activity modulations trigger robust polar state reversals of a macroscopic vortex formed by colloidal rollers. Here, we reveal that the shape anisotropy of dielectric rollers transforms the system into a chiral active fluid comprised of rollers of arbitrary handedness. The chiral rollers self-assemble into multiple freestanding vortices with a spontaneously selected sense of rotation. We demonstrate that upon reactivation of the system after a complete cessation of activity beyond all relevant timescales, the vortices simultaneously restore their previous chiral states in striking contrast to the chiral state reversals demonstrated by spherical rollers. The analysis reveals that shape-anisotropy modifies the collective state memory of the ensemble. The findings provide insights into the emergence of complex collective behavior in chiral colloidal fluids governed by an interplay between shape anisotropy, chiral motion, and activity modulations. Active chiral fluids exhibit the spontaneous emergence of correlated states, characterized by complex collective dynamics and self-organization. Shape anisotropy modifies the collective behavior of the active colloidal ensemble, enabling spontaneous restoration of chiral states across all self-organized vortices upon reactivation of the system.
Language: English
Open Access status: gold
Estimated APC paid: $3,990
OpenAlex ID: W4411164392
FWCI: 0.62
Cites: 57
Cited by: 2
Related to: 10