Synergistic control of radical generation in a radio-frequency atmospheric-pressure plasma jet via voltage waveform tailoring and structured electrodes
Year: 2025
Type: article
Abstract: The synergy between voltage waveform tailoring and structured electrodes is investigated in a radio -frequency atmospheric-pressure microplasma jet operated in helium with a 0.1% oxygen admixture. The device incorporates rectangular trenches in both electrodes and is driven by ‘Peaks’ and ‘Valleys’ waveforms synthesized from four harmonics (base frequency f b = 13.56 MHz, V pp = 500 V, and P = 1.2 W). Two-dimensional plasma fluid simulations, together with spatially and temporally resolved optical diagnostics (phase-resolved optical emission spectroscopy and tunable diode laser absorption spectroscopy), are used to demonstrate that the combination of asymmetric voltage waveforms with electrode structuring results in the strong spatial localization of electron power absorption and radical generation. This synergy leads to a single pronounced maximum inside a trench at either the powered or grounded electrode, depending on the applied waveform, unlike a symmetric excitation, which produces a spatially symmetric enhancement at both electrodes. This effect is attributed to the interplay between waveform-induced sheath dynamics and geometric focusing provided by the trenches, enabling electrically reversible and selective enhancement of electron power absorption at a chosen location.
Language: English
Subfield: Radiology, Nuclear Medicine and Imaging
Field: Medicine
Domain: Health Sciences
Open Access status: hybrid
Estimated APC paid: $3,325
Funder: Deutsche Forschungsgemeinschaft
Award: G554678873
OpenAlex ID: W4414317119
