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Microscale sensing with strongly interacting NV ensembles at high fields

Year: 2025
Type: article
Abstract: Advances in sensing devices that utilize nitrogen-vacancy (NV) center ensembles in diamond are driving progress in microscale nuclear magnetic resonance spectroscopy. Utilizing quantum sensing techniques in the high-field regime significantly boosts sensitivity by increasing thermal polarization and improves spectral quality via enhanced energy shifts. Compatible with the latter, a straightforward manner to further raise sensor sensitivity is to increase NV concentration, although this intensifies detrimental dipole-dipole interactions among NVs. In this Letter, we present a method for detecting NMR signals in high-field scenarios while effectively suppressing dipole-dipole couplings in the NV ensemble. Thus, this approach enhances sensitivity by combining highly doped diamond substrates and elevated magnetic fields.
Language: English
Open Access status: gold
Estimated APC paid: $2,625
OpenAlex ID: W4415260474
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Cites: 41
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