Work

Ferroelectrically controlled chirality switching of Weyl quasiparticles

Year: 2025
Type: article
Abstract: Weyl quasiparticles, as gapless low-energy excitations with nontrivial chirality, have garnered extensive interest in recent years. However, archieving effective and reversible control over their chirality (topological charge) remains a major challenge due to topological protection. In this Letter, we propose a ferroelectric mechanism to switch the chirality of Weyl phonons, where the reversal of ferroelectric polarization is intrinsically coupled to a simultaneous reversal of the chirality of Weyl points. This enables electric-field-driven control over the topological properties of phonon excitations. Through a comprehensive symmetry analysis of polar space groups, we identify 27 groups capable of hosting symmetry-protected Weyl phonons with chiral charges $C=1$, 2, and 3, whose chirality can be reversed via polarization switching. The first-principles calculations are performed to screen feasible material candidates for each type of chirality, yielding a set of prototypical ferroelectric compounds that realize the proposed mechanism. As a representative example, ${\mathrm{K}}_{2}{\mathrm{ZnBr}}_{4}$ hosts the minimal configuration of two pairs of Weyl phonons. Upon polarization reversal, the chirality of all Weyl points is inverted, accompanied by a reversal of associated topological features such as Berry curvature and surface arcs. These findings provide a viable pathway for dynamic, electrical control of topological band crossings and open different avenues for chirality-based phononic applications.
Language: English
Open Access status: green
OpenAlex ID: W4415348402
FWCI: 0.37
Cites: 101
Cited by: 1
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