Year: 2025
Type: article
Abstract: Optically active solid-state spin qubits thrive as an appealing technology for quantum interconnects and quantum networks, thanks to their atomic size, scalable synthesis, long-lived coherence, and ability to coherently interface with flying qubits. Trivalent erbium dopants, in particular, emerge as an attractive candidate due to their emission in the telecom C band and shielded 4f intra-shell spin and optical transitions. Nevertheless, prevailing top-down architectures for rare-earth qubits and devices have not yet achieved simultaneous long optical and spin coherence, which is necessary for efficient long-distance quantum networks. Here, we demonstrate dual Er3+ telecom spin-photon interfaces in two distinct lattice symmetry sites within an epitaxial thin-film platform. By leveraging high matrix crystallinity, controlled proximity of dopants to surfaces, and exploiting host lattice symmetry, we simultaneously achieve kilohertz-level optical linewidth in a strongly symmetry-protected site, and erbium qubit spin coherence times exceeding 10 milliseconds. Additionally, we realize single-shot readout and microwave coherent control of erbium qubits in a fiber-integrated package, enabling rapid deployment and scalability. These advancements highlight the significant potential of high-quality rare-earth qubits and quantum memories assembled using a bottom-up method, paving the way for scalable development of quantum light-matter interfaces tailored for telecommunication quantum networks. Erbium quantum emitters operating in the telecom C band are promising for spin-photon interfaces but achieving both optical and spin coherence has been challenging. Gupta et al. report two types of erbium dopants in epitaxial Y2O3 thin films occupying distinct lattice sites and exhibiting long spin and optical coherence times
Source: Nature Communications
Institutions: University of Chicago, University of Basel
Language: English
Subfield: Atomic and Molecular Physics, and Optics
Field: Physics and Astronomy
Domain: Physical Sciences
Open Access status: gold
Estimated APC paid: $6,990
Funders: National Science Foundation, U.S. Department of Defense, U.S. Department of Energy, Schweizerischer Nationalfonds zur Förderung der Wissenschaftlichen Forschung, U.S. Army, National Center of Competence in Research Quantum Science and Technology, Office of Naval Research, Division of Materials Research, Army Research Office, Argonne National Laboratory
Awards: Electro-optics of semiconductor nanostructures, G1917814032, CAREER:Long-distance quantum network of long-lived rare-earth qubits, Materials Research Science and Engineering Center, ENGINEERING RARE-EARTH HYPERFINE QUBITS FOR QUANTUM INFORMATION TECHNOLOGY, G4657484576, G4720003262, G5313541091, G6212337671, G628552264, G6671297155, PROGRAMMABLE ATOMIC ASSEMBLY OF OXIDES QUANTUM SYSTEMS USING MOLECULAR BEAM EPITAXY, G8048112891, G8876996369
OpenAlex ID: W4415958338
