Year: 2026
Type: article
Abstract: Chirality is a fundamental asymmetry in nature. In optics, control of chirality is evolving from spatial properties like polarization to the temporal chirality of local fields. Conventional approaches, however, encode chirality in abstract degrees of freedom such as phase or polarization, limiting direct and efficient coupling with matter on ultrafast timescales. We introduce and experimentally demonstrate a paradigm of intensity-driven optical chirality, where handedness is physically inscribed into the trajectory of spatiotemporal energy flow. Through the engineered non-collinear collision of Spatiotemporal Optical Vortices, the spatiotemporal optical coil is generated. The coil's chirality manifests as a physical torsion of its volumetric energy flow, a property distinct from chirality hidden in phase or polarization. By employing femtosecond tomography and phase-resolved reconstruction, we map the complete three-dimensional spatiotemporal intensity field, directly observing the evolution of singularity lines. This approach reveals programmable scaling relations between the coil's topology and interaction geometry, extending the concept of chirality to the energy-flow level. The introduced volumetric chiral density directly correlates with the optical forces and torques exerted on chiral particles, providing an intensity-manifested degree of freedom for topological photonics and enabling novel schemes for ultrafast chiral-selective excitation and high-dimensional information encoding.
Source: Light Science & Applications
Institutions: University of Shanghai for Science and Technology, Westlake University, Shanghai Jiao Tong University, Karlsruhe Institute of Technology, Fudan University, State Key Laboratory of Surface Physics, Yunnan Normal University, Paul Scherrer Institute, Freie Universität Berlin, Hiroshima University, International Institute for Sustainability with Knotted Chiral Meta Matter
Language: English
Subfield: Atomic and Molecular Physics, and Optics
Field: Physics and Astronomy
Domain: Physical Sciences
Open Access status: gold
Estimated APC paid: $4,190
OpenAlex ID: W4416440217
