Synergistic Modification of Cellulose Fibers With Graphene Oxide and Titanate Coupling Agent for Enhanced Natural Rubber Composites
Year: 2025
Type: article
Abstract: ABSTRACT Natural rubber (NR) requires reinforcement to overcome its inherent mechanical deficiencies, though conventional fillers face sustainability challenges. This study innovatively modifies cellulose fiber (CF)—a renewable resource—through synergistic treatment with graphene oxide (GO) and titanate coupling agent 201 (TCA201), aiming to enhance NR composite performance. Optimal results emerged at a 3:1 TCA201/CF ratio (TCA‐CF4), where TCA201/GO co‐modification (TCA‐CFG) demonstrated significant improvements: an 86.7% reduction in ΔG′, a 44.0% lower friction coefficient, alongside a 40.6% increased elongation at break and a 32.58% enhanced wet‐skid resistance versus unmodified CF composites. This dual‐modification strategy effectively addresses dispersion and interfacial bonding issues, offering an eco‐friendly approach for high‐performance NR composites.
DOI: 10.1002/app.70038
Authors: Wenhui Han, Mingchao Wang, Xiangxu Li, Chuansheng Wang, Huiguang Bian
Institution: Qingdao University of Science and Technology
Language: English
Subfield: Polymers and Plastics
Field: Materials Science
Domain: Physical Sciences
Open Access status: green
Awards: G1372840569, G861838046
OpenAlex ID: W4416534450
