Year: 2026
Type: article
Abstract: The combination of localized magnetic moments, their frustration and interaction with itinerant electrons is a key challenge of condensed matter physics. Frustrated magnetic interactions promote degenerate ground states with enhanced fluctuations, a topic that is predominantly studied in magnetic insulators. The coupling between itinerant and localized electrons in metals add complexity to the problem, and is presently formulated only for extreme cases in which the itinerant electrons mediate exchange between localized spins (RKKY interaction) or suppress the formation of magnetic moments (Kondo screening). Here, we report an in-depth experimental study of the distorted Kagome metal YbAgGe, unravelling the open questions of how frustration, localized magnetism and itinerant electrons are intertwined in frustrated Kondo metals. We find that coupled itinerant and localized electrons give rise to dynamic magnetic correlations below T * ≈ 20 K. At lower temperature, frustrated magnetic interactions establish anisotropic magnetic short-range correlations that culminate into antiferromagnetic long-range order below T N = 0.68 K with a significantly reduced modulated magnetic moment. We show that local moment Hamiltonians can yield limited understanding of the microscopic behaviour in frustrated metals, and prompt the extension of more sophisticated model Hamiltonians incorporating itinerant effects.
Source: Communications Materials
Language: English
Subfield: Condensed Matter Physics
Field: Physics and Astronomy
Domain: Physical Sciences
Open Access status: gold
Estimated APC paid: $3,690
Funders: National Science Foundation, U.S. Department of Energy, Iowa State University, Schweizerischer Nationalfonds zur Förderung der Wissenschaftlichen Forschung, Paul Scherrer Institut, Helmholtz-Zentrum Dresden-Rossendorf, Office of Science, Oak Ridge National Laboratory, Division of Materials Sciences and Engineering
Awards: G1418315740, G1519358529, G1866217153, G237429762, G2441759041, G249831736, Quantum Critical Phenomena in Metals with Competing Interactions, G333242795, Shadow Mineral and Rock Deformation Experiments at APS 6BM-B Beamline by Participants from ISRD-RCN, G498139845, G524707868, G5599649393, New structures and dynamics emerging from frustration, G5959670421, G628552264, G8943864594, G969889393, G993971353
OpenAlex ID: W4416708403
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