Electrically Tunable Ultraflat Bands and Ï -Electron Magnetism in Graphene Nanoribbons
Year: 2025
Type: article
Abstract: Atomically thin crystals hosting flat electronic bands have recently been identified as a rich playground for exploring and engineering strongly correlated phases. Yet, their variety remains limited, primarily to two-dimensional moire superlattices. Here, we predict the formation of reversible, electrically induced ultraflat bands and pi-electron magnetism in one-dimensional chevron graphene nanoribbons. Our ab initio calculations show that the application of a transverse electric field to these nanoribbons generates a pair of isolated, nearly perfectly flat bands with widths of approximately 1 meV around the Fermi level. Upon charge doping, these flat bands undergo a Stoner-like electronic instability, resulting in the spontaneous emergence of local magnetic moments at the edges of the otherwise nonmagnetic nanoribbon, akin to a one-dimensional spin-1/2 chain. Our findings expand the class of carbon-based nanostructures exhibiting flat bands and establish a novel route for inducing correlated electronic phases in chevron graphene nanoribbons.
Language: English
Subfield: Materials Chemistry
Field: Materials Science
Domain: Physical Sciences
Open Access status: green
OpenAlex ID: W6928801259
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