Observation of chiral phonons with giant magnetic moments in a topological crystalline insulator
Year: 2023
Type: article
Abstract: We have studied the magnetic response of transverse optical phonons in Pb1xSnxTe lms. Polarization-dependent terahertz magnetospectroscopy measurements revealed Zeeman splittings and diamagnetic shifts, demonstrating that these phonon modes become chiral in magnetic elds. Films in the topological crystalline insulator phase (x > 0:32) exhibited magnetic moment values that are larger than those for topologically trivial lms (x < 0:32) by two orders of magnitude. Furthermore, the sign of the eective g-factor was opposite in the two phases, a signature of the topological transition within our model. These results strongly indicate the existence of interplay between the magnetic properties of chiral phonons and the topology of electronic band structure.
Institutions: Universidade de São Paulo, Rice University, Yokohama National University, Tohoku University, Institute for Materials Research, Tohoku University, Instituto Nacional de Pesquisas Espaciais, Northeastern University, The University of Texas at Austin, Massachusetts Institute of Technology
Language: French
Subfield: Condensed Matter Physics
Field: Physics and Astronomy
Domain: Physical Sciences
Open Access status: green
Funders: National Science Foundation, Fundação de Amparo à Pesquisa do Estado de São Paulo, Conselho Nacional de Desenvolvimento Científico e Tecnológico, Materials Research Science and Engineering Center, Harvard University, Japan Society for the Promotion of Science, Division of Materials Research
Awards: G1372744343, G1500824199, G2680903639, Kerr/Faraday rotation in quantum materials, G2978038238, G4025248774, The research in new materials involving high magnetic fields and low temperatures, G4402799499, G4913504425, Center for Dynamics and Control of Materials, Development of Phase-Controlled Near Field Spectroscopy with Extremely High Spatiotemporal Resolution, G5719130415, G6725192607, G6796072035, Nonequilibrium Control of Magnetism and Topology Through Selective Phonon Excitations
OpenAlex ID: W6986155928
