Year: 2026
Type: article
Abstract: Air-sensitive 2D materials present fundamental challenges for device integration. Encapsulation is required to preserve intrinsic properties, yet conventional strategies require complicated fabrication workflows and fail with thicker flakes. We demonstrate that electron-beam (e-beam) evaporated aluminum oxide (AlOx) serves as an effective encapsulation layer and sacrificial fabrication mask, protecting sensitive flakes from air, photoresists, and chemicals. Unlike transfer-based approaches, this scalable technique requires no stacking and enables contacts without postencapsulation etching or harsh chemistry. Using rare-earth tritellurides (RTe3, R = La, Er), semimetallic WTe2, and superconducting FeTexSe1–x, we show that AlOx suppresses oxidation and preserves optical and electronic properties. We establish substrate-dependent optimization of encapsulation across a range of flake thicknesses, demonstrate that ultrathin AlOx preserves WTe2’s plasmonic response, and enhances superconducting performance in FeTexSe1–x devices when employed as a mask. Thus, we overcome the longstanding trade-off between encapsulation and straightforward device fabrication in fragile quantum materials.
Source: Nano Letters
Language: English
Subfield: Materials Chemistry
Field: Materials Science
Domain: Physical Sciences
Open Access status: hybrid
Estimated APC paid: $4,500
Funders: National Science Foundation, U.S. Department of Energy, Gordon and Betty Moore Foundation, Boston College, Fundação de Amparo à Pesquisa do Estado de São Paulo, Office of Science, Materials Research Science and Engineering Center, Harvard University, Division of Materials Research, Basic Energy Sciences, Air Force Office of Scientific Research
Awards: G119059943, G1662093594, G2034111186, G295657101, G3249401059, MRI: Acquisition of Thermal Scanning Probe Lithography in a Glovebox for Research and Training in Materials and Devices, G4516885165, G5326455407, G5363092874, G5592398945, G5596376502, Columbia University MRSEC on Precision-Assembled Quantum Materials, G5765906131, G5775595869, G6002429476, G6125720754, G6671297155, G6711204355, G6965541988, CAREER: QUANTUM MATERIALS IN SQUARE-NET BASED COMPOUNDS, G7453190137, G7463374569, G763802366, G7814707945, G9000849578, G9000850697, G9000851880
OpenAlex ID: W7204596384
FWCI:
Cites:
Cited by:
Related to:
