Work

Equilibrium and stability of soft-magnetic particle assemblies: A multipole model with polymer chain elasticity

Year: 2026
Type: article
Abstract: We present a discrete model for the equilibrium and stability of soft-magnetic particle-filled elastomers. The finite-sized spherical particles are tethered to the surrounding matrix or to neighboring particles by freely-jointed polymer chains with finite extensibility. The magnetic interactions are resolved through an approximate, self-consistent, saturating local-field magnetic dipole-dipole model augmented with dipole–quadrupole corrections. The latter become significant near contact, which is enforced through a simple Signorini contact model. The coupled magneto-elastic–contact problem is solved by two complementary strategies: an implicit arc-length continuation method that traces the complete equilibrium path, including unstable branches and limit points, and an explicit overdamped integrator that follows the physically realized loading and captures snap-through instabilities and the associated hysteresis. For two- and four-particle anchored assemblies, the model reveals three elementary regimes, i.e. repulsion, attraction, and repulsion-then-attraction. In turn, when extended to periodic body-centered-cubic arrays, the framework reveals collective particle chain formation and contact avalanches whose magnitude is governed by the compliance of the polymer chains. The additional dipole–quadrupole corrections leave global magnetization and the onset of bifurcation largely unchanged but increase the contact fraction and promote thicker particle-chain clustering near contact.
Language: English
Open Access status: hybrid
Estimated APC paid: $4,220
OpenAlex ID: W7212376984
FWCI:
Cites: 41
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Related to: 10