Year: 2026
Type: article
Abstract: Fallout radionuclide (FRN) archived in soils are key tracers of soil redistribution, sediment dynamics, and associated carbon fluxes, yet their global application is limited by poorly constrained baselines in the Southern Hemisphere. Here, we present the first hemisphere-scale baseline and uncertainty maps of 137 Cs and 239+240 Pu soil inventories. Predictions exhibited lower spatial variability and relative uncertaintyfor 137 Cs across most landscapes, whereas 239+240 Pu showed greater spatial variability and larger relative uncertainty. The reconstructed inventories revealed strong latitudinal and topographic gradients, with the highest predicted fallout occurring in tropical and mountainous regions. We further show, under a standardized hypothetical 50% inventory-loss scenario, that uncertainty in low-inventory regions can propagate nonlinearly into soil erosion and carbon-budget estimates, producing carbon budget biases of up to 19.8 t C ha −1 . These findings provide a new benchmark for Southern Hemisphere fallout radionuclide applications and a scalable framework for integrating spatial uncertainty into sediment tracing, soil degradation assessment, and carbon cycle studies.
Institutions: Bureau de Recherches Géologiques et Minières, University of Basel, Centre National de la Recherche Scientifique, Université de Versailles Saint-Quentin-en-Yvelines, Université Paris-Saclay, Laboratoire des Sciences du Climat et de l'Environnement, Laboratoire Environnements, Dynamiques et Territoires de Montagne, Université Savoie Mont Blanc, Université Grenoble Alpes, Institut polytechnique de Grenoble, Institut National de Recherche pour l'Agriculture, l'Alimentation et l'Environnement, Institut des Géosciences de l'Environnement, Institut de Recherche pour le Développement, Swiss Federal Institute for Forest, Snow and Landscape Research, ETH Zurich, Institute of Terrestrial Ecosystems
Language: English
Subfield: Pollution
Field: Environmental Science
Domain: Physical Sciences
SDGs: Life on land, Climate action
Open Access status: gold
Estimated APC paid: $3,490
OpenAlex ID: W7225428619
