Year: 2022
Type: preprint
Abstract: We demonstrate a 13-fold speed improvement in broadband cantilever-enhanced photoacoustic spectroscopy (CEPAS) by combining it with phase-controlled Fourier-transform spectroscopy (PC-FTS) instead of traditional Fourier-transform infrared spectroscopy (FTIR). PC-FTS is a modification of FTIR and capable of fundamentally faster interferogram acquisitions. The speed-improvement is beneficial for CEPAS, which is an especially sensitive version of the background-free photoacoustic spectroscopy technique. We used the PC-FTS-CEPAS technique to measure the absorption spectrum of methane in the mid-infrared region (3.3$-$3.5 $μ$m) with an optical frequency comb as the light source.
Source: arXiv (Cornell University)
Language: English
Subfield: Spectroscopy
Field: Chemistry
Domain: Physical Sciences
Open Access status: green
OpenAlex ID: W4312091024
