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LIFETIME OF THE METASTABLE 23S1 STATE IN STORED Li+ IONS

Year: 2010
Type: article
Abstract: A laser-induced fluorescence technique combined with the observation of spontane ous magnetic dipole photons from the highly metastable 2 3 S t state of Li + has been used to measure the radiative lifetime of this state.The ions are created by electron impact on a lithium A. Direct Determination of the Spontaneous Decay Curve .... 18 B. Direct Determination of the Number of Remaining Metastables 20 C. Indirect Determination of the Radiative Lifetime 23 IV.Ion Trap Theory and Performance 29 A. The RF-Quadrupole Ion Trap 29 B. The Ion Detection System 36 C. Ion Trap Performance 43 1.Ion storage 43 2. Ion distribution 50 V.Experimental Methods 56 A. The Vacuum System 56 B. The Lithium Oven and Hot Wire Detector 60 C. The Ion Trap and Electron Gun 62 D. The Magnetic Field 66 1. Detector operation ..... 73 2. Detector calibration 76 6.The Laser and Optical System 81 H.The Computer System 84 1. Timing and control .84 2. Operating and analysis programs 88 VI.Experimental Results 93 A. The Detection of Spontaneous Ml Photons 93 B. The Detection of Laser-Induced Photons 96 C. The Metastable Lifetime and Nonradiative Quenching .... 99 D. Procedures in Measuring the Radiative Lifetime 104 E. Data Reduction and Error Analysis Ill VII.Conclusion 119 Appendix A. Optical Pumping Calculations .121 A. The Magic Angle 121 B. The Optical Pumping Equations 123 C. Results of the Calculations .126 Appendix B. Measurements of the Ion Density Distribution 128 A. The Laser Scanning Technique 128 B. Experimental Results 130 Acknowledgements ....
Author: R. D. Knight
Language: English
Open Access status: green
OpenAlex ID: W800485256
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